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so I think I'm going to guess Amazing Adult Fantasy 1, which will be a milestone because it's the first double-size Masterworks.
That was my first thought too...fingers crossed!

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what's interesting about this is: This material has never been reprinted before, to my knowledge.(except the Hulk issues in Treasury format, among others)
I'm pretty sure both Marvel Premiere issues were reprinted in the Marvel Visionaries: Gil Kane TPB. I've never seen a copy of that book anywhere over the years, so I can't comment on the quality of the reproduction.