Since Iron Man V2 is (supposedly) in the pipeline, here is my Silver Age 10 Most Wanted List...

1) Avengers, V1: Avengers #1-31(including Avengers 1.5)
2) Ant-Man/Giant-Man and the Wasp: Tales to Astonish #27, 35-69 (including Wasp Tales),  story from Iron Man #44,  Marvel Feature #4-10, Marvel Team-Up #59-60,  Marvel Premiere #47-48, stories from Incredible Hulk Weekly #48-49
3) Thor, V1: Journey Into Mystery #83-120, Annual #1
(the beginning of Romita's run on) Spider-Man, V2: Amazing Spider-Man #39-67, Annuals #3-5
4) (Ditko's) Dr. Strange: Strange Tales #110, 111, 114-146, Amazing Spider-Man Annual #2
5) (the conclusion of Kirby's run on) Fantastic Four V3: Fantastic Four #61-102, Annual #5-6 and "The Lost" Lee-Kirby Story"
6) Captain America V1: Tales of Suspense #59-99, Captain America #100-113
7) Daredevil V1: Daredevil #1-32, Annual #1
8) Human Torch: Strange Tales #101-134, Strange Tales Annual #2, Marvel Team-Up # 1-3, 10, 18, 26, 29. 32, 35. 39, 47
9) Sub-Mariner V1: Tales to Astonish #70-101, Iron Man & Sub-Mariner #1, Sub-Mariner #1-13
10) either Thor V2 or S.H.I.E.L.D. V1